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Cubic optical nonlinearity of free electrons in bulk gold

N. I. Zheludev, P. J. Bennett, H. Loh, S. V. Popov, I. R. Shatwell, Yu. P. Svirko, V. E. Gusev, V. F. Kamalov, and E. V. Slobodchikov

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Abstract

A fast (τresponse <90 fs) free-electron spin-flipping frequency-degenerate nonlinearity with a significant value of ∣χxxyy(3)(ω,ω,ω,-ω)-χxyyx(3)(ω,ω,ω,-ω)∣~10-8 esu has been observed in bulk gold at 1260 nm by use of a new pump–probe polarization-sensitive technique.

© 1995 Optical Society of America

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