Abstract
We present time-resolved measurements of the electronic and the nuclear
contributions to the third-order nonlinearities of Ti:sapphire and
Cr:LiSGaF. The results suggest that nonlinear refraction in Ti:sapphire
is resonantly enhanced relative to that of undoped sapphire. The implications
of the nonlinear responses for short-pulse formation are discussed.
© 1998 Optical Society of America
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