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Fundamental limits on third-order molecular susceptibilities

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Abstract

By the use of sum rules, the largest third-order molecular nonlinear-optical susceptibilities allowed by quantum mechanics are determined. The theoretical upper limit is found to depend only on the first excited-state transition energy and on the number of electrons, in agreement with experimental data.

© 2000 Optical Society of America

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Corrections

Mark G. Kuzyk, "Fundamental limits on third-order molecular susceptibilities: erratum," Opt. Lett. 28, 135-135 (2003)
https://opg.optica.org/ol/abstract.cfm?uri=ol-28-2-135

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