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Nonlinear optical microscopy analysis of ultrafast phase transformation in vanadium dioxide

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Abstract

The nonlinear optical properties of solid–solid phase transformation in vanadium dioxide are studied. It is found that the efficiency of the third-harmonic optical signal generated from the surface of the material increases by 1.5 orders of magnitude as a function of this phase transformation. Microscopy studies show the hysteresis of the phase transformation on a micrometer-size scale.

© 2002 Optical Society of America

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