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Fourier transform measurement of two-photon excitation spectra: applications to microscopy and optimal control

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Abstract

We report a novel Fourier transform method for measuring two-photon excitation spectra. We demonstrate this method using simple dye molecules and discuss its applications in two-photon fluorescence microscopy and optimal control. This method facilitates an intuitive interpretation of recent control experiments in terms of tuning the nonlinear spectrum of the exciting laser source.

© 2005 Optical Society of America

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