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We calculate the spectrum of three-photon absorption (3PA) in zinc blende semiconductors using Kane’s four-band model. We apply this to ZnSe and measure the 3PA spectrum using femtosecond pulses, obtaining excellent agreement. The spectrum shows the apparent onset of 3PA from the split-off band and also shows quantum interference between the several possible evolution pathways when exciting carriers from valence to conduction band.
© 2008 Optical Society of America
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Claudiu M. Cirloganu, Peter D. Olszak, Lazaro A. Padilha, Scott Webster, David J. Hagan, and Eric W. Van Stryland, "Three-photon absorption spectra of zinc blende semiconductors: theory and experiment: erratum," Opt. Lett. 45, 1025-1026 (2020)https://opg.optica.org/ol/abstract.cfm?uri=ol-45-4-1025
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