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Pure rotational stimulated Raman photoacoustic spectroscopy

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Abstract

Pure rotational spectra of CO2 and N2O have been recorded by utilizing sensitive photoacoustic techniques to detect energy deposited in the gas sample as rotational excitation by stimulated Raman scattering. The unique features of this technique are its potential for high resolution and the complete absence of any signal that is due to Rayleigh scattering.

© 1979 Optical Society of America

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